Prof. Dr. Robert Schlögl - Heterogene Reaktionen

Vita

Diplom Maximilians Universität München (1979)
Dr. rer. nat. Maximilians Universität München (1982)
Postdoc Heterogeneous Catalysis, Cambridge University (Sir J. Meurig Thomas); Physics, Switzerland (Prof. H.J. Güntherodt) (1982 - 1983)
Gruppenleiter Hoffmann La Roche AG, Basel, Schweiz
Habilitation Structure of industrial ammonia-synthesis catalysts (Prof. Gerhard Ertl), FHI Berlin
Professor Inorganic Chemistry, Universität Frankfurt (1989 - 1994)
Direktor Fritz-Haber-Institut der MPG (seit 1994)
Honorarprofessor Technische Universität Berlin (seit 1994)
Honorarprofessor Humboldt-Universität Berlin (seit 1998)
Gründungs-Direktor MPI CEC (since 2011)
Honorarprofessor Universität Duisburg-Essen (seit 2013)
     
Vorträge

Liste aller Vorträge seit 1994

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Vorträge:

"Was tanken wir morgen?"
Vortrag am Infotag 'Synthetische Kraftstoffe - Optionen für eine nachhaltige Mobilität'
DECHEMA, 27.03.2019

Funktionen, Aufgaben & Preise

Funktionen & Aufgaben

  • Vice President of National Academy of Sciences Leopoldina (since 2020)
  • Member of National Hydrogen Council (since 2020)
  • Advisory Board Bavarian Battery Center at University Bayreuth (since 2020)
  • Supervisory Board of Helmholtz-Zentrum (2017)
  • Co-Chair SAPEA, CCU working group (2017)
  • Chairman Advisory Board “Kopernikusprojekte” of BMBF (since 2016)
  • Head of Steering Committee of “Energy Systems for the Future”, the academic advisory board to the German government (2012-2017)
  • Chair of Panel 4 (chemistry and Materials Sciences of the European Research Council) (2007-2010)
  • Fellow of the Royal Society of Chemistry, Cambridge, UK (2005)
  • Tetelman Fellow, Yale University, USA (2004)
  • President of the German Catalysis Society (1996-2003)

Preise & Auszeichnungen

  • 2020 Honorary Doctorate, Darmstadt University, Darmstadt
  • 2019 Ipatieff Lecturer
  • 2019 Eduard-Rhein-Kulturpreis
  • 2017 Ruhrpreis für Kunst und Wissenschaft der Stadt Mülheim a.d. Ruhr
  • 2017 ENI Award Energy Transition
  • 2016 Innovationspreis NRW
  • 2015 Alwin Mittasch Award
  • 2013 Max Planck Communitas Award
  • 2010 Dechema Medal
  • 1994 Otto Bayer Prize
  • 1989 Schunck Award for Innovative Materials

Editorship(s)

  • since 2009 ChemCatChem
  • since 2003 Catalysis Letters
  • 2003-2009 Journal of Catalysis
  • 1999-2003 Physical Chemistry-Chemical Physics
Publications

Full publications list

Selected MPI CEC publications

  • Tesch, M. F., Neugebauer, S., Narangoda, P. V., Schlögl, R.,  Mechler, A. K. (2023). The rotating disc electrode: measurement protocols and reproducibility in the evaluation of catalysts for the oxygen evolution reaction. ENERGY ADVANCES, 2(11), 1823-1830. doi:10.1039/d3ya00340j.
  • Blume, R., Calvet, W., Ghafari, A., Mayer, T., Knop-Gericke, A.,  Schögl, R. (2023). Structural and Chemical Properties of NiOx Thin Films: Oxygen Vacancy Formation in O-2 Atmosphere. ChemPhysChem, e202300231, pp. 1-11. doi:10.1002/cphc.202300231.
  • Rohner, C., Pratsch, C., Schlögl, R.,  Lunkenbein, T. (2023). Structural Identification and Observation of Dose Rate-Dependent Beam-Induced Structural Changes of Micro- and Nanoplastic Particles by Pair Distribution Function Analysis in the Transmission Electron Microscope (ePDF). Microscopy and Microanalysis, (29), 1566-1578. doi:10.1093/micmic/ozad087.
  • Mom, R. V., Sandoval-Diaz, L.-E., Gao, D., Chuang, C.-H., Carbonio, E. A., Jones, T. E., Arrigo, R., Ivanov, D., Hävecker, M., Roldan Cuenya, B., Schlögl, R., Lunkenbein, T., Knop-Gericke, A.,Velasco Vélez, J. (2023). Assessment of the Degradation Mechanisms of Cu Electrodes during the CO2 Reduction Reaction. ACS Applied Materials and Interfaces, (15), 30052-30059. doi:10.1021/acsami.2c23007.
  • Carbonio, E. A., Sulzmann, F., Klyushin, A. Y., Hävecker, M., Piccinin, S., Knop-Gericke, A., Schlögl, R., Jones, T. E. (2023). Adjusting the Chemical Reactivity of Oxygen for Propylene Epoxidation on Silver by Rational Design: The Use of an Oxyanion and Cl. ACS Catalysis, 13(9), 5906-5913. doi:10.1021/acscatal.3c00297.
  • Velasco-Velez, J. J., Poon, J., Gao, D., Chuang, C.-H., Bergmann, A., Jones, T. E., Haw, S.-C., Chen, J.-M., Carbonio, E., Mom, R. V., Ivanov, D., Arrigo, R., Cuenya, B. R., Knop-Gericke, A.,  Schlögl, R. (2023). Cationic Copper Species Stabilized by Zinc during the Electrocatalytic Reduction of CO2 Revealed by In Situ X-Ray Spectroscopy. Advanced Sustainable Systems, 2200453, pp. 1-7. doi:10.1002/adsu.202200453.
  • Esquius, J. R., Morgan, D. J., Siller, G. A., Gianolio, D., Aramini, M., Lahn, L., Kasian, O., Kondrat, S. A., Schlögl, R., Hutchings, G. J., Arrigo, R.,  Freakley, S. J. (2023). Lithium-Directed Transformation of Amorphous Iridium (Oxy)hydroxides To Produce Active Water Oxidation Catalysts. The Journal of Physical Chemistry A, (145), 6398-6409. doi:10.1021/jacs.2c13567.
  • Foppa, L., Rüther, F., Geske, M., Koch, G., Girgsdies, F., Kube, P., Carey, S. J., Hävecker, M., Timpe, O., V. Tarasov, A., Scheffler, M., Rosowski, F., Schlögl, R.,  Trunschke, A. (2023). Data-Centric Heterogeneous Catalysis: Identifying Rules and Materials Genes of Alkane Selective Oxidation. Journal of the American Chemical Society, (145), 3427-3442. doi:10.1021/jacs.2c11117.
  • Song, F., Straten, J. W., Lin, Y.-M., Ding, Y., Schlögl, R., Heumann, S., Mechler, A. K. (2023). Binder-Free N-Functionalized Carbon Electrodes for Oxygen Evolution Reaction. ChemElectroChem,(10) e202201075, pp. 1-10. doi:10.1002/celc.202201075.
  • Kube, P., Dong, J., Sanchez Bastardo, N., Ruland, H., Schlögl, R., Margraf, J. T., Reuter, K.,  Trunschke, A. (2023). Green synthesis of propylene oxide directly from propane. Nature Communications, 13(1): 7504, pp. 1-8. doi:10.1038/s41467-022-34967-2.
  • Klingenhof, M., Hauke, P., Kroschel, M., Wang, X., Merzdorf, T., Binninger, C., Thanh, T. N., Paul, B., Teschner, D., Schlögl, R., Strasser, P. (2022). Anion-Tuned Layered Double Hydroxide Anodes for Anion Exchange Membrane Water Electrolyzers: From Catalyst Screening to Performance. ACS Energy Letters, (7), 3415-3422. doi:10.1021/acsenergylett.2c01820.
  • Righi, G., Plescher, J., Schmidt, F.-P., Campen, R. K., Fabris, S., Knop-Gericke, A., Schlögl, R., Jones, T. E., Teschner, D., Piccinin, S. (2022). On the origin of multihole oxygen evolution in haematite photoanodes. Nature Catalysis, (5), 888-899. doi:10.1038/s41929-022-00845-9.
  • Kang, S., Im, C., Spanos, I., Schlögl, R., Ham, K., Lim, A., Jacobs, Timo , Lee, Jaeyoung (2022). Durable Nickel-Iron (Oxy)hydroxide Oxygen Evolution Electrocatalysts through Surface Functionalization with Tetraphenylporphyrin. (61): e202214541, pp. 1-10. doi:10.1002/anie.202214541.
  • Žeradjanin, A. R., Narangoda, P., Masa, J.,  Schlögl, R. (2022). What Controls Activity Trends of Electrocatalytic Hydrogen Evolution Reaction?-Activation Energy Versus Frequency Factor. ACS CATALYSIS, (19), 11597-11605. doi:10.1021/acscatal.2c02964.
  • Ghampson, I. T., Lundin, S.-T.-B., Vargheese, V., Kobayashi, Y., Huff, G. S., Schlögl, R., Trunschke, A.,  Oyama, S. T. (2022). Methane selective oxidation on metal oxide catalysts at low temperatures with O2 using an NO/NO2 oxygen atom shuttle. Journal of Catalysis, (408), 401-412. doi:10.1016/j.jcat.2021.07.014.
  • Streibel, V., Velasco-Velez, J. J., Teschner, D., Carbonio, E. A., Knop-Gericke, A., Schlögl, R.,  Jones, T. E. (2022). Merging operando and computational X-ray spectroscopies to study the oxygen evolution reaction. Current Opinion in Electrochemistry, (35) 101039,  doi:10.1016/j.coelec.2022.101039.
  • Choudhury, S. H., Ding, Y., Yi, Y., Rohner, C., Frandsen, W., Lunkenbein, T., Greiner, M., Schlögl, R., Heumann, S. (2022). Oxidation Behavior of Glassy Carbon in Acidic Electrolyte. ChemElectroChem, (9): e202200637, pp. 1-7. doi:10.1002/celc.202200637.
  • Deerberg, G., Oles, M., Schlögl, R. (2022). Carbon2Chem (R) - A Key Building Block for Climate Protection. SI, 94(10), 1387-1387. doi:10.1002/cite.202271002.
  • Türk, H., Götsch, T., Schmidt, F.-P., Hammud, A., Ivanov, D., de Haart, L. G. J., Vinke, I. C., Eichel, R.-A., Schlögl, R., Reuter, K., Knop-Gericke, A., Lunkenbein, T.,  Scheurer, C. (2022). Sr Surface Enrichment in Solid Oxide Cells - Approaching the Limits of EDX Analysis by Multivariate Statistical Analysis and Simulations. ChemCatChem, (14): e202200300, pp. 1-13. doi:10.1002/cctc.202200300.
  • Hegen, O., Salazar Gomez, J. I., Gruenwald, C., Rettke, A., Sojka, M., Klucken, C., Pickenbrock, J., Filipp, J., Schlögl, R.,  Ruland, H. (2022). Bridging the Analytical Gap Between Gas Treatment and Reactor Plants in Carbon2Chem (R). CHEMIE INGENIEUR TECHNIK, (94), 1405-1412. doi:10.1002/cite.202200015.
  • Ristig, S., Poschmann, M., Folke, J., Gomez-Capiro, O., Chen, Z., Sanchez-Bastardo, N., Schlögl, R., Heumann, S.,  Ruland, H. (2022). Ammonia Decomposition in the Process Chain for a Renewable Hydrogen Supply. Chemie-Ingenieur-Technik, (94), 1413-1425. doi:10.1002/cite.202200003.
  • Lin, Y., Yu, L., Tang, L., Song, F., Schlögl, R., Heumann, S. (2022). In Situ Identification and Time-Resolved Observation of the Interfacial State and Reactive Intermediates on a Cobalt Oxide Nanocatalyst for the Oxygen Evolution Reaction. ACS Catalysis, 12(9), 5345-5355. doi:10.1021/acscatal.1c05598.
  • Haase, F. T., Rabe, A., Schmidt, F.-P., Herzog, A., Jeon, H. S., Frandsen, W., Narangoda, P. V., Spanos, I., Ortega, K. F., Timoshenko, J., Lunkenbein, T., Behrens, M., Bergmann, A., Schlögl, R.,  Cuenya, B. R. (2022). Role of Nanoscale Inhomogeneities in Co2FeO4 Catalysts during the Oxygen Evolution Reaction. Journal of the American Chemical Society, 144(27), 12007-12019. doi:10.1021/jacs.2c00850.
  • Papakonstantinou, G., Spanos, I., Dam, A. P., Schlögl, R., Sundmacher, K. (2022). Electrochemical evaluation of the de-/re-activation of oxygen evolving Ir oxide. PHYSICAL CHEMISTRY CHEMICAL PHYSICS, 24(23), 14579-14591. doi:10.1039/d2cp00828a.
  • Sandoval-Diaz, L. E., Schlögl, R., Lunkenbein, T. (2022). Quo Vadis Dry Reforming of Methane?-A Review on Its Chemical, Environmental, and Industrial Prospects. Catalysts, 12(5): 465. doi:10.3390/catal12050465.
  • Schlögl, R. (2022). Interfacial catalytic materials; challenge for inorganic synthetic chemistry. ZEITSCHRIFT FUR NATURFORSCHUNG SECTION B-A JOURNAL OF CHEMICAL SCIENCES, (xx), xx-xx. doi:10.1515/znb-2022-0070.
  • Velasco Vélez, J., Bernsmeier, D., Jones, T. E., Zeller, P., Carbonio, E., Chuang, C.-H., Falling, L. J., Streibel, V., Mom V, R., Hammud, A., Hävecker, M., Arrigo, R., Stotz, E., Lunkenbein, T., Knop-Gericke, A., Krähnert, R.,  Schlögl, R. (2022). The rise of electrochemical NAPXPS operated in the soft X-ray regime exemplified by the oxygen evolution reaction on IrOx electrocatalysts. Faraday Discussions, (236), 103-125. doi:10.1039/d1fd00114k.
  • Kenmoe, S., Douma, D. H., Raji, A. T., M'Passi-Mabiala, B., Goetsch, T., Girgsdies, F., Knop-Gericke, A., Schlögl, R.,  Spohr, E. (2022). X-ray Absorption Near-Edge Structure (XANES) at the O K-Edge of Bulk Co3O4: Experimental and Theoretical Studies. Nanomaterials, 12(6): 921, pp. 1-10. doi:10.3390/nano12060921.
  • Codeco, C. F. S., Klyushin, A. Y., Carbonio, E. A., Knop-Gericke, A., Schlögl, R., Jones, T., Rocha, T. C. R. (2022). Insights into the electronic structure of hydroxyl on Ag(110) under near ambient conditions. Physical Chemistry Chemical Physics, 24(15), 8832-8838. doi:10.1039/d1cp02929k.
  • Schlögl, R. (2022). Chemical Batteries with CO2. Angewandte Chemie, International Edition in English, (61): e202007397, pp. 1-23. doi:10.1002/anie.202007397.
  • Arrigo, R., Blume, R., Streibel,V., Genovese, C., Roldan, A., Schuster, M. E., Ampelli, C., Perathoner, S., Velasco Vélez, J., Hävecker, M., Knop-Gericke, A., Schlögl, R.,  Centi, G. (2022). Dynamics at Polarized Carbon Dioxide-Iron Oxyhydroxide Interfaces Unveil the Origin of Multicarbon Product Formation. ACS Catalysis, (12), 411-430. doi:10.1021/acscatal.1c04296.
  • Hegen, O., Salazar Gomez, J. I., Schlögl, R., Ruland, H. (2022). The potential of NO+ and O-2(+center dot) in switchable reagent ion proton transfer reaction time-of-flight mass spectrometry. Mass Spectrometry Reviews, e21770. doi:10.1002/mas.21770.
  • Folke, J., Dembele, K., Girgsdies, F., Song, H., Eckert, R., Reitmeier, S., Reitzmann, A., Schlögl, R., Lunkenbein, T., Ruland, H. (2022). Promoter effect on the reduction behavior of wuestite-based catalysts for ammonia synthesis. Catalysis Today, (387) 12-22. doi:10.1016/j.cattod.2021.03.013.
  • Wang, Y., Rosowski, F., Schlögl, R., Trunschke, A. (2022). Oxygen Exchange on Vanadium Pentoxide. The Journal of Physical Chemistry C, 126(7), 3443-3456. doi:10.1021/acs.jpcc.2c00174.
  • Lange, T., Reichenberger, S., Ristig, S., Rohe, M., Strunk, J., Barcikowski, S., Schlögl, R. (2022). Zinc sulfide for photocatalysis: White angel or black sheep? Progress in Materials Science, 124: 100865. doi:10.1016/j.pmatsci.2021.100865.
  • Sanchez-Bastardo, N., Schlögl, R.,  Ruland, H. (2021). Response to Comment on "Methane Pyrolysis for Zero-Emission Hydrogen Production: A Potential Bridge Technology from Fossil Fuels to a Renewable and Sustainable Hydrogen Economy". Industrial and Engineering Chemistry Research, 60(48), 17795-17796. doi:10.1021/acs.iecr.1c04435.
  • Schlögl, R. (2021). Chemical Batteries with CO2. Angewandte Chemie, International Edition in English, (60), 2-25. doi:10.1002/anie.202007397.
  • Dreyer, M., Cruz, D., Hagemann, U., Zeller, P., Heidelmann, M., Salamon, S., Landers,J., Rabe,A., Ortega,K.F. , Najafishirtari,S., Wende,H., Hartmann,N., Knop-Gericke,A., Schlögl,R., Behrens,M.  (2021) The Effect of Water on the 2-Propanol Oxidation Activity of Co-Substituted LaFe1-CoxO3 Perovskites. SI, (27) 17127 - 17144 doi:10.1002/chem.202102791.
  • Narangoda, P., Spanos, I., Masa, J., Schlögl, R., Zeradjanin, A. R. (2021) Electrocatalysis Beyond 2020: How to Tune the Preexponential Frequency Factor. ChemElectroChem, (8), 1-9. doi:10.1002/celc.202101278.
  • Schlögl, R. (2021) Material Science for catalysis: Quo vadis? Zeitschrift für anorganische und allgemeine Chemie, (647) 1998-2000. doi:10.1002/zaac.202100277.
  • Ronge, E., Ohms, J., Roddatis, V., Jones, T., Sulzmann, F., Knop-Gericke, A., Schlögl. R., Kurz, P.,Jooss, C., Skorupska, K. (2021) Operation of calcium-birnessite water-oxidation anodes: interactions of the catalyst with phosphate buffer anions. Sustainable Energy & Fuels, (5) 5535-5547. doi:10.1039/d1se01076j.
  • Koch, G., Hävecker, M., Kube, P., Tarasov, A., Schlögl, R., Trunschke, A. (2021). The Influence of the Chemical Potential on Defects and Function of Perovskites in Catalysis. Frontiers in Chemistry, 9, 746229-746229. doi:10.3389/fchem.2021.746229.
  • Zeradjanin, A. R., Narangoda, P., Spanos, I., Masa, J.,  Schlögl, R. (2021). How to minimise destabilising effect of gas bubbles on water splitting electrocatalysts? CURRENT OPINION IN ELECTROCHEMISTRY, 30: 100797. doi:10.1016/j.coelec.2021.100797.
  • Salazar Gomez, J. I., Sojka, M., Klucken, C., Schlögl, R.,  Ruland, H. (2021). Determination of trace compounds and artifacts in nitrogen background measurements by proton transfer reaction time-of-flight mass spectrometry under dry and humid conditions. Journal of Mass Spectrometry, 56(8): e4777, pp. 1-22. doi:10.1002/jms.4777.
  • Sanchez-Bastardo, N., Schlögl, R.,  Ruland, H. (2021). Methane Pyrolysis for Zero-Emission Hydrogen Production: A Potential Bridge Technology from Fossil Fuels to a Renewable and Sustainable Hydrogen Economy. INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH, 60(32), 11855-11881. doi:10.1021/acs.iecr.1c01679.
  • Türk, H., Schmidt, F. P., Götsch, T., Girgsdies, F., Hammud, A., Ivanov, D., Vinke, I.,de Haart, L.G.J.,Eichel, R.A., Reuter, K., Schlögl, R., Knop-Gericke, A., Scheurer, C., Lunkenbein, T. (2021). Complexions at the Electrolyte/Electrode Interface in Solid Oxide Cells. Advanced Materials Interfaces, 8 (18): 2100967, pp. 1-9. doi:10.1002/admi.202100967.
  • Ronge, E., Ohms, J., Roddatis, V., Jones, T., Sulzmann, F., Knop-Gericke, A., Schlögl, R., Kurz, P., Jooss, C., Skorupska, K. (2021). Operation of calcium-birnessite water-oxidation anodes: interactions of the catalyst with phosphate buffer anions. Sustainable Energy & Fuels (5) 5535-5547. doi:10.1039/d1se01076j.
  • Foppa, L., Ghiringhelli, L. M., Girgsdies, F., Hashagen, M., Kube, P., Hävecker, M., Carey, S., Tarasov, A., Kraus, P., Rosowski, F., Schlögl, R., Trunschke, A., Scheffler, M. (2021) Materials genes of heterogeneous catalysis from clean experiments and artificial intelligence. MRS Bulletin (46) 1016-1026. doi:10.1557/s43577-021-00165-6.
  • Velasco Vélez, J., Carbonio, E. A., Chuang, C.-H., Hsu, C.-J., Lee, J.-F., Arrigo, R., Hävecker, M., Wang, R., Plodinec, M., Wamg, F.R., Centeno, A., Zurutuza, A., Falling, L.J., Mom, V., Hofmann, S., Schlögl, R., Knop-Gericke, A., Jones, T.,(2021). Surface Electron-Hole Rich Species Active in the Electrocatalytic Water Oxidation. Journal of the American Chemical Society, 143(32) 12524-12534 . doi:10.1021/jacs.1c01655.
  • Zeradjanin, A. R., Narangoda, P., Spanos, I., Masa, J., Schlögl, R. (2021). Expanding the frontiers of hydrogen evolution electrocatalysis & ndash;searching for the origins of electrocatalytic activity in the anomalies of the conventional model. ELECTROCHIMICA ACTA, 388: 138583. doi:10.1016/j.electacta.2021.138583.
  • Schlögl, R. (2021). Quo vadis carbocatalysis? Journal of Energy Chemistry, 61, 219-227. doi:10.1016/j.jechem.2021.02.024.
  • Hausmann, J. N., Schlögl, R., Menezes, P. W.,  Driess, M. (2021). Is direct seawater splitting economically meaningful? Energy & Environmental Science, (14), 3679-3685. doi:10.1039/d0ee03659e.
  • Hartwig, C., Schweinar, K., Jones, T. E., Beeg, S., Schmidt, F.-P., Schlögl, R., Greiner, M . (2021). Isolated Pd atoms in a silver matrix: Spectroscopic and chemical properties. The Journal of Chemical Physics, 154(18): 184703, pp. 1-10. doi:10.1063/5.0045936.
  • Fan, H., Folke, J., Liu, Z., Girgsdies, F., Ruland, H., Imlau, R., Ruland,H., Heumann, S., Granwehr, J., Eichel,R.- A., Schlögl, R., Frei, E.,Xing, H. (2021) Ultrathin 2D Fe-Nanosheets Stabilized by 2D Mesoporous Silica: Synthesis and Application in Ammonia Synthesis. ACS Appl. Mater. Inerfaces, 13(25), 30187-30197. doi:10.1021/acsami.1c06771
  • Huang, X., Jones, T., Federov, A., Farra, R., Coperet, C., Schlögl, R., Willinger,M.-G. (2021). Phase Coexistence and Structural Dynamics of Redox Metal Catalysts Revealed by Operando TEM. Advanced Materials,(33) 2101772, pp. 1-11. doi:10.1002/adma.202101772.
  • Ding, Y., Zhang, L., Gu, Q., Spanos, I., Pfänder, N., Wu, K. H., Schlögl, R., Heumann, S. (2021). Tuning of Reciprocal Carbon-Electrode Properties for an Optimized Hydrogen Evolution. ChemSusChem, 14(12), 2547-2553. doi:10.1002/cssc.202100654.
  • Pielsticker, L., Nicholls, R., Beeg, S., Hartwig, C., Klihm, G., Schlögl, R., Tougaard, S., Greiner, M.(2021). Inelastic electron scattering by the gas phase in near ambient pressure XPS measurements. Surface and Interface Analysis, (53) 605-617. doi:10.1002/sia.6947.
  • Chee, S. W., Lunkenbein, T., Schlögl, R., Cuenya, B. R. (2021). In situ and operando electron microscopy in heterogeneous catalysis-insights into multi-scale chemical dynamics. Journal of Physics: Condensed Matter, 33(15): 153001, pp. 1-28. doi:10.1088/1361-648X/abddfd.
  • Lange, T., Reichenberger, S., Rohe, M., Bartsch, M., Kampermann, L., Klein, J., Schlögl, R.,  Barcikowski, S. (2021). Alumina-Protected, Durable and Photostable Zinc Sulfide Particles from Scalable Atomic Layer Deposition. Advanced Functional Materials, 31(14): 2009323, pp. 1-15. doi:10.1002/adfm.202009323.
  • Schlögl, R. (2021). Chemical energy storage enables the transformation of fossil energy systems to sustainability. Green Chemistry, 23(4), 1584-1593. doi:10.1039/d0gc03171b.
  • Zeradjanin, A. R., Masa, J., Spanos, I., Schlögl, R. (2021). Activity and Stability of Oxides During Oxygen Evolution Reaction---From Mechanistic Controversies Toward Relevant Electrocatalytic Descriptors. Frontiers in Energy Research, 8, 613092. https://doi:10.3389/fenrg.2020.613092.
  • Nong, H. N., Falling, L. J., Bergmann, A., Klingenhof, M., Tran, H. P., Spori, C., Mom, R., Timoshenko, J., Zichittella, G., Knop-Gericke, A., Piccinin, S., Perez-Ramirez, J., Cuenya, B. R., Schlögl, R., Strasser, P., Teschner, D., Jones, T. E. (2021). Key role of chemistry versus bias in electrocatalytic oxygen evolution (vol 587, pg 408, 2020). Nature, E8. https://www.nature.com/articles/s41586-020-03141-3.pdf
  • Spanos, I., Masa, J., Zeradjanin, A., Schlögl, R. (2021). The Effect of Iron Impurities on Transition Metal Catalysts for the Oxygen Evolution Reaction in Alkaline Environment: Activity Mediators or Active Sites? Catalysis Letters 151, 1843-1856 https://doi.org/10.1007/s10562-020-03478-4
  • Klingenhof, M., Hauke, P., Brückner, S., Dresp, S., Wolf, E., Nong, H.N., Spöri, Merzdorf, T., Bernsmeier, D., Teschner, D., Schlögl, R., Strasser, P. (2021). Modular Design of Highly Active Unitized Reversible Fuel Cell Electrocatalysts ACS Energy Letters 6(1), 177-183.   https://doi.org/10.1021/acsenergylett.0c02203
  • Ruiz Esquius, J., Algara-Siller, G., Spanos, I., Freakley, S.J., Schlögl, R., Hutchings, G.J. (2020). Preparation of Solid Solution and Layered IrOx–Ni(OH)2 Oxygen Evolution Catalysts: Toward Optimizing Iridium Efficiency for OER ACS Catalysis 10(24), 14640-146448. https://doi.org/10.1021/acscatal.0c03866
  • Boniface, M., Plodinec, M., Schlögl, R., Lunkenbein, T. (2020). Quo Vadis Micro-Electro-Mechanical Systems for the Study of Heterogeneous Catalysts Inside the Electron Microscope? Topics in Catalysis 63(15-18), 1623-1643. https://doi.org/10.1007/s11244-020-01398-6
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  • Buller, S., Heise-Podleska, M., Pfänder, N., Willinger, M., Schlögl, R. (2016). Carbon nanotubes as conducting support for potential Mn-oxide electrocatalysts: Influences of pre-treatment procedures Journal of Energy Chemistry 25(2), 265-271. https://doi.org/10.1016/j.jechem.2016.01.022
  • Lee, J., Eiswirth, M., Schlögl, R. (2016). Preface: Surface analysis and dynamics Catalysis Today, 260, 1-2. https://doi.org/10.1016/j.cattod.2015.10.008
  • Maganas, D., Trunschke, A., Schlögl, R., Neese, F. (2016). A unified view on heterogeneous and homogeneous catalysts through a combination of spectroscopy and quantum chemistry Faraday Discussions 188, 181-197. https://doi.org/10.1039/c5fd00193e
  • Arrigo, R., Schuster, M.E., Abate, S., Giorgianni, G., Centi, G., Perathoner, S., Wrabetz, S., Pfeifer, V., Antonietti, M., Schlögl, R. (2016). Pd Supported on Carbon Nitride Boosts the Direct Hydrogen Peroxide Synthesis ACS Catalysis 6(10), 6959-6966. https://doi.org/10.1021/acscatal.6b01889
  • Mette, K., Kühl, S., Tarasov, A., Willinger, M.-G., Kröhnert, J., Wrabetz, S., Trunschke, A., Scherzer, M., Girgsdies, F., Düdder, H., Kähler, K., Ortega, K.F., Muhler, M., Schlögl, R., Behrens, M., Lunkenbein, T. (2016). High-Temperature Stable Ni Nanoparticles for the Dry Reforming of Methane ACS Catalysis 6(10), 7238-7248. https://doi.org/10.1021/acscatal.6b01683
  • Klyushin, A.Y., Greiner, M.T., Huang, X., Lunkenbein, T., Li, X., Timpe, O., Friedrich, M., Hävecker, M., Knop-Gericke, A., Schlögl, R. (2016). Is Nanostructuring Sufficient To Get Catalytically Active Au? ACS Catalysis 6(5), 3372-3380. https://doi.org/10.1021/acscatal.5b02631
  • Schlögl, R. (2016). Sustainable Energy Systems: The Strategic Role of Chemical Energy Conversion Topics in Catalysis 59(8-9), 772-786. https://doi.org/10.1007/s11244-016-0551-9
  • Pfeifer, V., Jones, T.E., Velasco-Vélez J.J., Massué, C., Arrigo, R., Teschner, D., Girgsdies, F., Scherzer, M., Greiner, M.T., Allan, J., Hashagen, M., Weinberg, G., Piccinin, S., Hävecker, M., Knop-Gericke, A., Schlögl, R. (2016). The electronic structure of iridium and its oxides Surface and Interface Analysis 48(5), 261-273. https://doi.org/10.1002/sia.5895
  • Schumann, J., Tarasov, A., Thomas, N., Schlögl, R., Behrens, M. (2016). Cu,Zn-based catalysts for methanol synthesis: On the effect of calcination conditions and the part of residual carbonates Applied Catalysis A - General 516, 117-126. https://doi.org/10.1016/j.apcata.2016.01.037
  • Pfeifer, V., Jones, T.E., Velasco-Vélez, J.J., Massué, C., Greiner, M.T., Arrigo, R., Teschner, D., Girgsdies, F., Scherzer, M., Allan, J., Hashagen, M., Weinberg, G., Piccinin, S., Hävecker, M., Knop-Gericke, A., Schlögl, R. (2016). The electronic structure of iridium oxide electrodes active in water splitting Physical Chemistry Chemical Physics 18(4), 2292-2296. https://doi.org/10.1039/c5cp06997a 
  • Pfeifer, V., Jones, T.E., Wrabetz, S., Massué, C., Velasco-Vélez, J.J., Arrigo, R., Scherzer, M., Piccinin, S., Hävecker, M., Knop-Gericke, A., Schlögl, R. (2016). Reactive oxygen species in iridium-based OER catalysts Chemical Science 7(11), 6791-6795. https://doi.org/10.1039/c6sc01860b
Abteilungsmitglieder

Wissenschaftliche Mitarbeiter*innen

Dr. Raoul Blume
Dr. Michael Hävecker
Dr. Benjamin Johnson
Dr. Yang-Ming Lin
Dr. Justus Masa
Dr. Marc Müller
Dr. Garlef Wartner
Dr. Aleksandar Zeradanin

Postdocs

Dr. Zongkun Chen
Dr. Sayed Mahmoud Elrefaei
Dr. Jan Markus Folke
Dr. Christian Froese
Dr. Christoph Göbel
Dr. Oscar Gómez-Cápiro
Dr. Kahyun Ham
Dr. Elisabeth Hannah Hetaba-Wolf
Dr. Jacob Johny
Dr. Daniel Laudenschleger
Dr. Ahyoun Lim
Dr. Clara Markert
Dr. Tammarat Niemeier
Dr. Lukas Pielsticker
Dr. Corina Helene Pollok
Dr. Michael Poschmann
Dr. Daniela Ramermann
Dr. Simon Ristig
Dr. Marc Tesch
Dr. Sebastian Tigges
Dr. Wenchao Wan

PhD Studierende

Liseth Johana Duarte Correa
Melina Müller

Labor

Sandra Denner
Alina-Denise Ernst
Dennis Ernst
Marius Heise-Podleska
Natalia Jakobs
Janina Jaspert
Christian Klucken
Lea Kreutzheide
John-Tommes Krzeslack
Dieter Oppenberg
Norbert Pfänder
Alin Benice Schöne
Martha Sojka
Teresa Stamm
Agnes Stoer
Johanna Taing
Miriam van den Höövel
Lars Weber

Heterogeneous Reactions

The energy challenge can be seen as the major challenge for today’s society and future generations. Chemistry plays a central role in the energy challenge, since most energy conversion systems work on (bio)chemical energy carriers and require for their use suitable process and material solutions. The enormous scale of their application demands optimization beyond the incremental improvement of empirical discoveries. For this reason we work on the development of knowledge-based systematic approaches in order to arrive at scalable and sustainable solutions.

Analysis of the processes that are essential to convert the current energy systems into sustainable systems indicates that the conversion of electricity into chemical energy is a critical process in the network of chemical energy conversion reactions. Both electrolysis and heterogeneous photochemical reactions are of relevance here. The difficult elementary steps are in the oxygen evolution reaction.

In a concerted effort the department develops a concept of carbon-based functional materials that operate in oxygen evolution either alone or doped with functional transition metal oxides. In parallel we study with advanced in-situ spectroscopic tools the reaction on performing systems with noble metals to learn about design requirements for systems operating with materials as used in the biological analogue. The resulting material solutions and synthesis tools will be transferred to catalytic processes binding primary hydrogen onto carrier molecules such as CO2 and N2 to arrive at practically useful solar fuels.

The work of the department is strictly knowledge-oriented to generate generic insight and solutions for synthesis and analysis of chemical energy conversion systems. Theory and molecular model studies with the other departments critically deepen our insight. The department engages into method development for operating advanced spectroscopic methods on heterogeneous and on homogeneous systems. Projects are performed in close collaboration with the Fritz-Haber-Institute of the Max Planck Society in Berlin.